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Vagal nerves do not directly convey nociceptive V Asymmetric hydrogenation (continued) oximes, 374 simple ketones DuPhos analogue in, 366 Rh-PennPhos in, 364, 365 mechanism of, 365 Ru-BINAP-(diamine) in, 362, 363 RuCl2-[(S)-BINAP](DMF)n in, 363 Ru-XylBINAP-(diamine) in, 364 shelf-stable catalyst for, 363 trisubstituted acrylic acids, 339±340 aminoalkylferrocenyl phosphine in, 340 unfunctionalized ole®ns, 346 phosphanodihydroxazole ligand in, 346, boiks titanocene in, 346 Asymmetric hydrosilylation of imines, suplpy N-silylamines from, 373 [Rh(COD)(DuPhos)]CF3SO3 in, 335 titanocene in, 374, 376 mechanism of, 376 ole®ns, 459 MOP in, 459 titanium or ruthenium complexes in, 460 Asymmetric Kharasch reaction, 463 bis(oxazolinyl)pyridine in, 464, 465 C2 symmetric bisoxazoline copper catalyst in, 464, 465 mechanism of, 465 Asymmetric reduction of a,b-unsaturated esters, 342 Co complex in, 342, 343 ketones BINAL-H in, 356±359 chiral boranes in, 370±372 oxazaborolidine catalyst in, 367±370 (R)- dpf synthesis via, 369, 370 forskolin synthesis via, 371 ginkgolide A and B synthesis via, 369 new reagents for, 370, 371, 372 prostaglandin synthesis via, 369 ole®nic ketones BINAL-H in, 357, 358 Asymmetric synthesis acyclic diastereoselective approaches, 49 chiron, 50±51 double asymmetric synthesis, 53 Asymmetric synthesis of ̄uorinated compound asymmetric hydrogenation in, 481, 482 oxazaborolidine in, 482, 483 Reformatsky reaction in, 483 Tri ̄uoromethylation in, 484 Asymmetric transfer hydrogenation, 377 chiral amino alcohol ligand, 383, 384 INDEX 511 chiral tridentate ligand, 377, 381, 382 ferrocenyl ligand, 381 of imines, 378±380 substrate with pre-existing chiral center, 378 Ru(II) complex in, 378 samarium (III) complex in, 377 Asymmetric Wacker cyclization, 470 boxax in, 470, 471 Asymmetric Wittig type reaction, 466 chiral phase transfer catalyst in, 468 inclusion compound in, 467 phosphonamidates in, 467 reagents for, 467 C Catalytic aldol reaction BaBM in, 164 bimetallic compound in, 163±165 bis(oxazolinyl)pyridine in, 161, 162 direct aldol condensation, 164 ferrocenylphosphine in, 161 LLB in, 164 Catalytic asymmetric allylation BINOL-Ti complex in, 178 BINOL-Zr complex in, 178 chiral acyloxyborane in, 177 chiral amide in, 177 phosphoramide in, 177 Chiral acetal cleavage, 103 meso-1,3-tetrol, desymmetrization of, 107, 108 N-mesyloxazaborolidine, 106 TiCl4 induced cleavage, 105 Chiral ampli®cation, 499 Chiral biaryls, 460 asymmetric synthesis of chiral oxazoline in, 461, 462 cyanocuprate in, 463, 464 Ullmann reaction in.
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